Alexandre Pato will join Villarreal from Corinthians after an unsuccessful loan spell at Chelsea last season.
Barcelona have signed former Manchester City prospect Denis Suarez on a four-year contract from Villarreal.
Denis Cheryshev has returned to former club Villarreal after completing his move from Real Madrid.
Manchester United have confirmed the signing of Ivory Coast centre-back Eric Bailly from Villarreal, subject to a work permit.
Villarreal defender Eric Bailly has passed a medical at Manchester United, according to Sky sources.
Villarreal were crowned champions as Spain's top young talent competed at the La Liga Promises tournament.
Manchester United are in talks with Villarreal to sign Ivory Coast international Eric Bailly, according to Sky sources.
All you need to know about Ivory Coast defender Eric Bailly, who has signed for Manchester United.
Fast and easy online Sky Sports upgrade
Watch the action with a Sky Sports Pass
Free to play! Pick your team today
Check out all the latest transfer news
Prize draws every day until August 14